Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Technical note: Sensitivity of the CAMS regional air quality modelling system to anthropogenic emission temporal variability
Marc Guevara,Augustin Colette,Antoine Guion,Valentin Petiot,Mario Adani,Joaquim Arteta,Anna Benedictow,Robert Bergström,Andrea Bolignano,Paula Camps,Ana C. Carvalho,Jesper Heile Christensen,Florian Couvidat,Ilia D’Elia,Hugo Denier van der Gon,Gaël Descombes,John Douros,Hilde Fagerli,Yalda Fatahi,Elmar Friese,Lise Frohn,Michael Gauss,Camilla Geels,Risto Hänninen,Kaj Hansen,Oriol Jorba,Jacek W. Kaminski,Rostislav Kouznetsov,Richard Kranenburg,Jeroen Kuenen,Victor Lannuque,Frédérik Meleux,Agnes Nyíri,Yuliia Palamarchuk,Carlos Pérez García-Pando,Lennard Robertson,Felicita Russo,Arjo Segers,Mikhail Sofiev,Joanna Struzewska,Renske Timmermans,Andreas Uppstu,Alvaro Valdebenito,and Zhuyun Ye
Abstract. An accurate characterization of the temporal distribution in primary emissions is essential for air quality modeling. This study evaluates the impact of replacing the default temporal profiles in the Copernicus Atmosphere Monitoring Service (CAMS) European air quality multi-model ensemble with an updated dataset (CAMS-REG-TEMPO). The sensitivity of 11 regional models and the ensemble to these changes is assessed by comparing modeled and observed monthly, weekly, and diurnal cycles of nitrogen dioxide (NO2), ozone (O3), coarse particulate matter (PM10), and fine particulate matter (PM2.5) across Europe. NO2 shows the greatest improvement, with weekly cycle correlations increasing up to +0.17 due to better road transport emissions representation. PM10 correlations improve in winter (up to +0.13 weekly and +0.07 diurnal) due to refined residential wood combustion emissions. PM2.5 correlations remain largely unchanged, except for diurnal cycles, which improve in winter (+0.18) but slightly degrade in spring and summer (-0.02). O3 is the least affected, as correlations were already high with default profiles (0.9–0.95). For some species and timescales (e.g., NO2 diurnal cycles), results vary across models, highlighting the complex interactions between emission timing and atmospheric processes. CAMS-REG-TEMPO has little effect on annual RMSE and bias, aside from slight improvements in high PM10 concentrations. Overall, the findings support implementing CAMS-REG-TEMPO in the operational CAMS multi-model ensemble.
Received: 18 Mar 2025 – Discussion started: 11 Apr 2025
Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this preprint. The responsibility to include appropriate place names lies with the authors.
Air quality models require hourly emissions to accurately represent dispersion and physico-chemical processes in the atmosphere. Since emission inventories are typically provided at the annual level, emissions are downscaled to a refined temporal resolution using temporal profiles. This study quantifies the impact of using new anthropogenic temporal profiles on the performance of an European air quality multi-model ensemble. Overall, the findings indicate an improvement of the modelling results.
Air quality models require hourly emissions to accurately represent dispersion and...