Preprints
https://doi.org/10.5194/egusphere-2023-1096
https://doi.org/10.5194/egusphere-2023-1096
07 Aug 2023
 | 07 Aug 2023

Sensitivity of global direct aerosol radiative forcing to uncertainties in aerosol optical properties

Jonathan Elsey, Nicolas Bellouin, and Claire Ryder

Abstract. New satellite missions promise global reductions in the uncertainties of aerosol optical properties but it is unclear how those reductions will propagate to uncertainties in the shortwave direct aerosol radiative effect (DARE) and radiative forcing (DARF), which are currently large, on the order of at least 20 %. In this work we build a Monte-Carlo framework to calculate the impact of uncertainties in aerosol optical depth (AOD), single scattering albedo (SSA) and asymmetry parameter on the uncertainty in shortwave DARE and DARF. This framework uses the results of over 2.3 million radiative transfer simulations to calculate global clear-sky DARE and DARF based on a range of aerosol optical property uncertainties, representative of existing and future global observing systems. We find the one-sigma uncertainty varies between ±0.23 to ±1.91 Wm-2 (5 and 42 %) for the top of atmosphere (TOA) clear-sky DARE and between ±0.08 to ±0.47 Wm-2 (9 and 52 %) for the TOA DARF. At the TOA, AOD uncertainty is the main contributor to overall uncertainty, except over bright surfaces where SSA uncertainty contributes most. We apply regionally varying uncertainties to represent current measurement uncertainties, finding that aerosol optical property uncertainties represent 24 % of TOA DARE and DARF. Reducing regionally varying optical property uncertainties by a factor of two would reduce their contributions to TOA DARE and DARF uncertainty proportionally. Scaling to all-sky conditions, aerosol optical property uncertainty contributes to about 25 % total uncertainty in TOA, all-sky DARE and DARF. Compared to previous studies which considered uncertainties in non-aerosol variables, our results suggest that the aerosol optical property uncertainty accounts for a third to a half of total uncertainty. Recent and future progress in constraining aerosol optical properties using ground-based or satellite retrievals could be translated into DARE and DARF uncertainty using our freely available framework.

Jonathan Elsey et al.

Status: final response (author comments only)

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2023-1096', Anonymous Referee #1, 11 Sep 2023
  • RC2: 'Comment on egusphere-2023-1096', Stefan Kinne, 13 Sep 2023

Jonathan Elsey et al.

Data sets

Radiative effect and forcing sensitivity data and software Jonathan Elsey, Nicolas Bellouin, Claire Ryder https://doi.org/10.5281/zenodo.7958296

Jonathan Elsey et al.

Viewed

Total article views: 397 (including HTML, PDF, and XML)
HTML PDF XML Total Supplement BibTeX EndNote
269 114 14 397 28 10 12
  • HTML: 269
  • PDF: 114
  • XML: 14
  • Total: 397
  • Supplement: 28
  • BibTeX: 10
  • EndNote: 12
Views and downloads (calculated since 07 Aug 2023)
Cumulative views and downloads (calculated since 07 Aug 2023)

Viewed (geographical distribution)

Total article views: 382 (including HTML, PDF, and XML) Thereof 382 with geography defined and 0 with unknown origin.
Country # Views %
  • 1
1
 
 
 
 
Latest update: 10 Dec 2023
Download
Short summary
Aerosols influence the Earth’s Energy balance. The uncertainty in this radiative forcing is large, depending partly on uncertainty in measurements of aerosol optical properties. We develop a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty but that non-aerosol uncertainties must also be considered.