the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
30 years of total column ozone and aerosol optical depth measurements using the Brewer spectrophotometer in Poprad-Gánovce, Slovakia
Abstract. Long-term measurement series are a rare but valuable source of information. The first measurements using the Brewer ozone spectrophotometer in Slovakia began at the Poprad-Gánovce station in August 1993. As a result, a 30-year series of measurements was completed in 2023. The primary goal of this study is to present the calculated values of total column ozone (TCO) and aerosol optical depth (AOD) derived from measurements conducted with the same Brewer spectrophotometer. Additionally, this time series of measurements is enriched with tropopause height values, made possible by aerological sounding measurements regularly conducted at the Poprad-Gánovce station. This work provides a climatological and long-term trend analysis of the time series for these three atmospheric characteristics. The data used in this study are closely tied to three environmental issues driven by human activities: ozone depletion, climate change, and air pollution caused by aerosols. No clear trend was observed for the annual TCO averages, while AOD at 320 nm exhibited a distinct decresing trend with a slope of −0.06 per decade. The lowest annual average of AOD at 320 nm was measured in 2020, corresponding to the first year of the COVID-19 pandemic. The highest increases in tropopause height were found in August, at 200 m per decade, and in September, at 210 m per decade. The largest declines in TCO occurred in the same months, with a rate of change of −3.5 DU per decade in August and −2.8 DU per decade in September.
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RC1: 'Good 30 years time series. Expand on tropopause height and total column ozone.', Anonymous Referee #1, 11 Jul 2025
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The manuscript presents 30 years of total column ozone and aerosol optical depth data measured by a Brewer Spectrometer at the Poprad Ganovce station in Slovakia, in Eastern Europe. In addition, tropopause height data are presented from regular radiosonde lauches at the same site. In large parts, the paper is an update of a previous paper by Hrabčák et al. (2018), which uses the same instrument and methods. The authors report a significant decreasing trend of aerosol optical depth, in all seasons, a significant increasing trend in tropopause height, throughout most of the year, and little or no trend in total column ozone.
Consistent long-term observations, like the ones present here, are important and deserve publication in a journal like ACP. While the manuscript presents no ground-braking new results, it still confirms findings of other studies, and helps with our understanding of long-term changes in the atmosphere. I suggest publication in ACP after a few generally minor revisions.
Section 2.4, in my opinion is rather lengthy, difficult to understand, and essentially a complete repeat of what is already presented in Hrabčák et al. (2018). I suggest to remove most of section 2.4, only describe the most salient points, and otherwise refer to Hrabčák et al. (2018). Essentially, to get aerosol optical depth, you need the measured intensity S from the Brewer, the ETC S_0, and you have to subtract ozone and Rayleigh optical depths times their air-masses. Why not write the relevant Equation that provides aerosol optical depth, and then say that Hrabčák et al. (2018) explain how to get all the parameters in that Equation. If there is anything different from Hrabčák et al. (2018), then explain that. Doing this will reduce Section 2.4 from about 100 lines to 10 or 20 lines, and will make the manuscript much more readable.
Figure 2: you might want to show another panel, which would present the annual cycle of tropopause height in a similar fashion. You might be surprised how closely the annual cycle of tropopause height mirrors the annual cycle of total column ozone.
Lines 286 to 292: I would drop this paragraph. It is not needed here.
Tables 3 to 6: It would be good to have additional columns giving uncertainty estimates for the trends.
Figure 6 and Table 6: It would be very interesting to see hypothetical TCO time series and trends, in which the -11.6 DU/km "dependence" on tropopause height has been backed out. Such a hypothetical time series in Fig. 6 might show a TCO increase, and the hypothetical effect of tropopause height changes. In Table 6, the hypothetical TCO trends would mostly become more positive by around 1 DU / decade. In fact, an additional Figure showing the seasonal variation of TCO trend, tropopause height related TCO trend and "hypothetical" TCO trend would be interesting. I suggest that the authors add such a Figure and discuss it. The slightly positive "hypothetical" TCO trend would be inline with ozone increases expected to to declining ODS (possibly enhanced by stronger Brewer Dobson Circulation). The discussion would give more meaning and context for tropopause height / climate change influences on total column ozone, and would round the paper nicely.
Citation: https://doi.org/10.5194/egusphere-2025-2887-RC1
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