Preprints
https://doi.org/10.5194/egusphere-2024-3911
https://doi.org/10.5194/egusphere-2024-3911
28 Feb 2025
 | 28 Feb 2025

Measurement report: Number size distribution of sub-40 nm particles in the Amazon rainforest

Jianqiang Zhu, Guo Li, Uwe Kuhn, Bruno Backes Meller, Christopher Pöhlker, Paulo Artaxo, Ulrich Pöschl, Yafang Cheng, and Hang Su

Abstract. The Amazon rainforest is a unique environment to investigate aerosol properties with limited impact from human activities, further providing a new perspective to look at the aerosol characteristics in regions heavily affected by anthropogenic emissions. Obtaining the size distributions of nucleation mode particles in the atmosphere is key to understanding aerosol formation, evolution and their impacts. Although routine and long-term aerosol measurements have been conducted in the Amazon region, information regarding sub-10 nm particles is still limited. In this study, we performed aerosol measurements from December 2022 to January 2023 on a 54-meterhigh platform of the Amazon Tall Tower Observatory (ATTO). Three advanced instruments namely the Nano Condensation Nuclei Counter (nCNC), the Neutral Cluster and Air Ion Spectrometer (NAIS), and the NanoScanning Mobility Particle Sizer (SMPS), were employed to measure the number size distributions of aerosol particles and naturally charged ions smaller than 40 nm. The results reveal that the median total number concentration of the measured particles with diameters ranging from 1.5 nm to 1000 nm was 969 cm-3. We found concentration. There was a significant increase in the number concentration of sub-3 nm particles in January 2023 (median, 573 cm-3) a large number of particles smaller than 3.5 nm, which accounted for up to 59 % of the measured total number compared to December 2022 (371 cm-3). The median number concentration of particles above 3.5 nm in December and January were 481 and 335 cm-3, respectively. No typical regional new particle formation events were observed throughout the measurement period. However, clear diurnal variations were observed for the sub-3 nm particles under pristine conditions, with the maximum concentration around noontime. Similar diurnal patterns were also observed for natural cluster ions (0.8–2 nm), with their concentration in January slightly higher than in December. Quantifying the properties of the aerosol particles in the Amazon rainforest helps to understand the processes governing the aerosol budget in the pristine atmosphere, and is essential for determining the impact of anthropogenic aerosols on climate.

Competing interests: At least one of the (co-)authors is a member of the editorial board of Atmospheric Chemistry and Physics.

Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this paper. While Copernicus Publications makes every effort to include appropriate place names, the final responsibility lies with the authors. Views expressed in the text are those of the authors and do not necessarily reflect the views of the publisher.
Share
Jianqiang Zhu, Guo Li, Uwe Kuhn, Bruno Backes Meller, Christopher Pöhlker, Paulo Artaxo, Ulrich Pöschl, Yafang Cheng, and Hang Su

Status: final response (author comments only)

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2024-3911', Anonymous Referee #1, 24 Mar 2025
    • AC1: 'Reply on RC1', Jianqiang Zhu, 25 Jul 2025
  • RC2: 'Comment on egusphere-2024-3911', Anonymous Referee #2, 15 Apr 2025
    • AC2: 'Reply on RC2', Jianqiang Zhu, 25 Jul 2025
Jianqiang Zhu, Guo Li, Uwe Kuhn, Bruno Backes Meller, Christopher Pöhlker, Paulo Artaxo, Ulrich Pöschl, Yafang Cheng, and Hang Su

Data sets

Measurement report: Number size distribution of sub-40 nm particles in the Amazon rainforest Jianqiang Zhu, Guo Li, Uwe Kuhn, Bruno Backes Meller, Christopher Pöhlker, Paulo Artaxo, Ulrich Pöschl, Yafang Cheng, and Hang Su https://doi.org/10.17617/3.ZBHLIR

Jianqiang Zhu, Guo Li, Uwe Kuhn, Bruno Backes Meller, Christopher Pöhlker, Paulo Artaxo, Ulrich Pöschl, Yafang Cheng, and Hang Su

Viewed

Total article views: 482 (including HTML, PDF, and XML)
HTML PDF XML Total Supplement BibTeX EndNote
376 90 16 482 38 18 41
  • HTML: 376
  • PDF: 90
  • XML: 16
  • Total: 482
  • Supplement: 38
  • BibTeX: 18
  • EndNote: 41
Views and downloads (calculated since 28 Feb 2025)
Cumulative views and downloads (calculated since 28 Feb 2025)

Viewed (geographical distribution)

Total article views: 488 (including HTML, PDF, and XML) Thereof 488 with geography defined and 0 with unknown origin.
Country # Views %
  • 1
1
 
 
 
 
Latest update: 08 Sep 2025
Download
Short summary
The manuscript reports unique measurement data on sub-40 nm particles and ions, especially those smaller than 10 nm in the Amazon from December 2022 to January 2023. A large number of sub-3 nm particles and naturally charged ions were present in the Amazonia boundary layer, and they showed a clear diurnal variation. The research will contribute to a better understanding of atmospheric processes in the pristine environment.
Share