the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Evaluating CHASER V4.0 global formaldehyde (HCHO) simulations using satellite, aircraft, and ground-based remote sensing observations
Abstract. Formaldehyde (HCHO), a precursor to tropospheric ozone, is an important tracer of volatile organic compounds (VOCs) in the atmosphere. Two years of HCHO simulations obtained from the global chemistry transport model CHASER at a horizontal resolution of 2.8° × 2.8° have been evaluated using observations from the Tropospheric Ozone Monitoring Experiment (TROPOMI), Atmospheric Tomography Mission (ATom), and multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations. CHASER reproduced the observed global HCHO spatial distribution with a spatial correlation (r) of 0.93 and a negative bias of 7 %. The model showed good capability for reproducing the observed magnitude of the HCHO seasonality in different regions, including the background conditions. The discrepancies between the model and satellite in the Asian regions were related mainly to the underestimated and missing anthropogenic emission inventories. TROPOMI's finer spatial resolution than that of the Ozone Monitoring Experiment (OMI) sensor reduced the global model–satellite root-mean-square-error (RMSE) by 20 %. The OMI and TROPOMI observed seasonal variations in HCHO abundances were consistent. However, the simulated seasonality showed better agreement with TROPOMI in most regions. The simulated HCHO and isoprene profiles correlated strongly (R = 0.81) with the ATom observations. CHASER overestimated HCHO mixing ratios over dense vegetation areas in South America and the remote Pacific (background condition) regions, mainly within the planetary boundary layer (< 2 km). The simulated temporal (daily and diurnal) variations in the HCHO mixing ratio showed good congruence with the MAX-DOAS observations and agreed within the 1-sigma standard deviation of the observed values.
Status: open (until 20 May 2024)
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CEC1: 'Comment on egusphere-2024-734', Juan Antonio Añel, 28 Mar 2024
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Dear authors,
Unfortunately, after checking your manuscript, it has come to our attention that it does not comply with our "Code and Data Policy".
https://www.geoscientific-model-development.net/policies/code_and_data_policy.htmlIn your manuscript, the "Code Availability" section says that the code relevant for your manuscript is only available under request to authors. The policy of Geosc. Model Dev. (which you should have read and complied with before submitting your manuscript) is very strict and clear, all the code and data relevant for a manuscript must be available in a public repository of the ones listed in our policy before submission.
Therefore, if you do not fix promptly this problem, we will reject your manuscript for publication in our journal. I should note that, given this lack of compliance with our policy, your manuscript should not have been accepted in Discussions.
Therefore, please, publish your code and in one of the appropriate repositories, and reply to this comment with the relevant information (link and DOI). This includes the MAX-DOAS data.
Also, you must include in a potentially reviewed version of your manuscript the modified 'Code Availability' and 'Data Availability' sections, with links and DOIs.
Juan A. Añel
Geosci. Model Dev. Executive EditorCitation: https://doi.org/10.5194/egusphere-2024-734-CEC1 -
AC1: 'Reply on CEC1', H.M.S. Hoque, 29 Mar 2024
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Dear Chief Editor,
Thank you very much for pointing out the issue. As the corresponding author, I take responsibility for the unintentional mistake. The model source code is accessible through https://zenodo.org/records/10892945 (Sudo et al., 2024), and the MAX-DOAS data is accessible through https://zenodo.org/records/10052384 (Hoque et al., 2024). Here is the revised code and data availability statement, which will be included in the revised version of the manuscript.
Code availability: The CHASER source code needed to reproduce the simulations in this work is available from the repository at https://zenodo.org/records/10892945 (Sudo et al., 2024).
Data availability: The processed model output and observational datasets needed to reproduce the results are available from the repository at https://zenodo.org/records/10052384 (Hoque et al., 2024). The MAX-DOAS profile and column data provided by Dr. Hitoshi Irie can be accessed from the repository(i.e., Hoque et al., 2024). TROPOMI (https://scihub.copernicus.eu/dhus/#/home, last access: 01 July 2023; De Smedt et al., 2021), OMI BIRA product, (https://www.temis.nl/qa4ecv/hcho/hcho_omi.php, last access: 01 July 2023; De Smedt et al., 2021) and ATom(https://daac.ornl.gov/ATOM/guides/ATom_nav.html, last access: 01 July 2023; Wofsy et al., 2018) data were obtained from the respective websites.
Reference:
Hoque, H. M. S., Sudo, K., and Irie, H., Model and observational datasets used for evaluating CHASER simulated formaldehyde (HCHO) abundances in 2019 and 2020. [Dataset]. Zenodo. https://doi.org/10.5281/zenodo.10052384, 2024
Sudo, K.: Evaluating CHASER V4.0 global formaldehyde (HCHO) simulations using satellite, aircraft, and ground-based remote sensing observations.[Dataset].Zenodo https://zenodo.org/records/10892945
Kind Regards,
Syedul Hoque
Citation: https://doi.org/10.5194/egusphere-2024-734-AC1
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AC1: 'Reply on CEC1', H.M.S. Hoque, 29 Mar 2024
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RC1: 'Comment on egusphere-2024-734', Anonymous Referee #1, 15 Apr 2024
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The comment was uploaded in the form of a supplement: https://egusphere.copernicus.org/preprints/2024/egusphere-2024-734/egusphere-2024-734-RC1-supplement.pdf
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