Preprints
https://doi.org/10.5194/egusphere-2026-3261
https://doi.org/10.5194/egusphere-2026-3261
07 Jul 2026
 | 07 Jul 2026

Ozone Downward Flux Revealed by High-Resolution Differential Absorption Lidar over Tibet during Stratosphere-Troposphere Exchange

Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li

Abstract. This study characterizes a prominent ozone intrusion event driven by STE that occurred on 18–19 October 2017. The analysis is enabled by high spatiotemporal resolution ozone profile observations from the USTC Ozone Lidar deployed at Yangbajing, Tibet (29° N, 99° E). It provides the first lidar-based detection of these rapid ozone descent events and the evidence linking them to temperature variability in the tropopause region through lidar-derived temperature profiles, revealing temperature gradients that generally exceed 8 K km−1 during these events and beyond the resolving capability of conventional atmospheric model products. Combining Wei’s flux diagnostic with a sensitivity test of PV-based dynamical tropopause thresholds identifies 3 PVU as the most suitable definition for this case. ERA5 is then used to characterize the spatiotemporal evolution of cross-tropopause mass fluxes over 25–28° N, 95–99° E, showing that the ozone variations observed by the lidar were modulated by gravity waves associated with the tropopause fold. In addition, lidar-measured ozone profiles are incorporated into a cross-tropopause ozone flux calculation framework, yielding an instantaneous peak STE ozone flux of about 3~4·10-10·kg·s-1·m-2, slightly higher than the corresponding ERA5 value, while maintaining strong agreement in overall flux magnitude and temporal evolution throughout the event. These results show that high-resolution vertical ozone observations and Raman-retrieved temperature profiles from the USTC Ozone Lidar, combined with wind field data, enable accurate quantification of STE-related ozone fluxes. This approach facilitates in-depth investigation of coupled atmospheric composition and dynamical processes.

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Journal article(s) based on this preprint

17 Sep 2026
Ozone downward flux revealed by high-resolution differential absorption lidar over Tibet during stratosphere-troposphere exchange
Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li
Atmos. Chem. Phys., 26, 13139–13156, https://doi.org/10.5194/acp-26-13139-2026,https://doi.org/10.5194/acp-26-13139-2026, 2026
Short summary
Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • CC1: 'use of Wei method to estimate STE', Heini Wernli, 14 Jul 2026
    • AC1: 'Reply on CC1', Ruichun Dong, 28 Jul 2026
  • RC1: 'Comment on egusphere-2026-3261', Anonymous Referee #1, 29 Jul 2026
  • RC2: 'Comment on egusphere-2026-3261', Anonymous Referee #2, 30 Jul 2026
  • CC2: 'Comment on egusphere-2026-3261', D. C. Wu, 05 Aug 2026
    • AC5: 'Reply on CC2', Ruichun Dong, 21 Aug 2026
  • RC3: 'Comment on egusphere-2026-3261', Anonymous Referee #3, 06 Aug 2026

Peer review completion

AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Ruichun Dong on behalf of the Authors (21 Aug 2026)  Author's response   Author's tracked changes   Manuscript 
ED: Referee Nomination & Report Request started (31 Aug 2026) by Bernd Funke
RR by Anonymous Referee #1 (01 Sep 2026)
RR by Anonymous Referee #2 (01 Sep 2026)
RR by Anonymous Referee #3 (04 Sep 2026)
ED: Publish subject to minor revisions (review by editor) (04 Sep 2026) by Bernd Funke
AR by Ruichun Dong on behalf of the Authors (06 Sep 2026)  Author's response   Author's tracked changes   Manuscript 
ED: Publish as is (07 Sep 2026) by Bernd Funke
AR by Ruichun Dong on behalf of the Authors (08 Sep 2026)  Manuscript 

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • CC1: 'use of Wei method to estimate STE', Heini Wernli, 14 Jul 2026
    • AC1: 'Reply on CC1', Ruichun Dong, 28 Jul 2026
  • RC1: 'Comment on egusphere-2026-3261', Anonymous Referee #1, 29 Jul 2026
  • RC2: 'Comment on egusphere-2026-3261', Anonymous Referee #2, 30 Jul 2026
  • CC2: 'Comment on egusphere-2026-3261', D. C. Wu, 05 Aug 2026
    • AC5: 'Reply on CC2', Ruichun Dong, 21 Aug 2026
  • RC3: 'Comment on egusphere-2026-3261', Anonymous Referee #3, 06 Aug 2026

Peer review completion

AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Ruichun Dong on behalf of the Authors (21 Aug 2026)  Author's response   Author's tracked changes   Manuscript 
ED: Referee Nomination & Report Request started (31 Aug 2026) by Bernd Funke
RR by Anonymous Referee #1 (01 Sep 2026)
RR by Anonymous Referee #2 (01 Sep 2026)
RR by Anonymous Referee #3 (04 Sep 2026)
ED: Publish subject to minor revisions (review by editor) (04 Sep 2026) by Bernd Funke
AR by Ruichun Dong on behalf of the Authors (06 Sep 2026)  Author's response   Author's tracked changes   Manuscript 
ED: Publish as is (07 Sep 2026) by Bernd Funke
AR by Ruichun Dong on behalf of the Authors (08 Sep 2026)  Manuscript 

Journal article(s) based on this preprint

17 Sep 2026
Ozone downward flux revealed by high-resolution differential absorption lidar over Tibet during stratosphere-troposphere exchange
Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li
Atmos. Chem. Phys., 26, 13139–13156, https://doi.org/10.5194/acp-26-13139-2026,https://doi.org/10.5194/acp-26-13139-2026, 2026
Short summary
Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li
Ruichun Dong, Xin Fang, Chengyun Yang, and Tao Li

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The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.

Short summary
High-resolution USTC Ozone Lidar observations at Yangbajing, Tibet capture short-lived rapid STE-related ozone descent for the first time. Lidar temperature profiles link these events to tropopause thermal variability unresolved by conventional models. Wei’s flux diagnostic and PV-threshold sensitivity identify 3 PVU as optimal. ERA5 shows gravity-wave modulation during tropopause folding, and lidar ozone profiles are used to quantify instantaneous cross-tropopause ozone flux.
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