Electrostatics and Collision Dynamics of Ice and Anthropogenic Smoke Particles in the Mesosphere/Lower Thermosphere
Abstract. The increase in satellite launches raises the anthropogenic influx of various elements into the Mesosphere and Lower Thermosphere (MLT), comparable to the natural influx caused by meteoric ablation. This study investigates the electrostatic interactions between ice particles and remnants of space debris using a classical electrostatic framework. Aside from the Coulomb interaction, the attractive force between two particles at short distances, arising from polarization, is taken into account. Collision outcomes, the effective velocity regime for collisions, and the subsequent aggregation probability are estimated. Aggregation is limited to a specific range of collision velocities between minimum and maximum values. This range varies depending on factors such as particle size, mass density, and dielectric constant. For most particles, the aggregation velocities range from a few m s-1 to several tens of m s-1, where smaller particles may need significantly higher velocities to form stable aggregates. When considering the collisions of particles in thermal motion, it is found that Al2O3 (due to its greater abundance) and TiO2 (due to its higher dielectric constant), both originating from anthropogenic sources, may dominate in the formation of ice-anthropogenic particle aggregates. In the MLT region, the formation of stable aggregates from the collision of ice with particles from space debris, which one may denote as anthropogenic smoke particles (ASPs), is similar to that from collisions with meteoric smoke particles (MSPs).
This manuscript applies a classical electrostatic theory to the collision and aggregation of charged mesospheric ice particles with anthropogenic smoke particles (ASPs) originating from re-entering space debris, deriving the minimum and maximum relative velocities that permit stable aggregate formation. The authors then use this to show that abundant or high-dielectric anthropogenic oxides such as Al₂O₃ and TiO₂ are likely to dominate aggregate formation, an interesting finding that can tell experimentalists what to look for. The study is timely and clearly written, and I recommend publication after consideration of the following minor comments.
Minor comments