Preprints
https://doi.org/10.5194/egusphere-2026-2896
https://doi.org/10.5194/egusphere-2026-2896
06 Jul 2026
 | 06 Jul 2026
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Observations of radiocarbon (14C) in atmospheric CO2 confirm decline in U.S. emissions of fossil fuel CO2 (FFCO2) between 2010 and 2015

S. M. Nazrul Islam, Scott J. Lehman, Sourish Basu, Arlyn E. Andrews, Kathryn McKain, Colm Sweeney, Xiaomei Xu, Chad Wolak, Stephen P. Morgan, Patrick Cappa, John R. Southon, Pieter P. Tans, and John B. Miller

Abstract. All emissions pathways aimed at stabilizing global temperatures at the internationally agreed target of 1.5–2 °C above pre-industrial levels require steep cuts in global CO2 emissions. Reliable emissions tracking is therefore essential to monitoring progress towards related mitigation goals, especially for the world’s largest emitters. Here we make use of atmospheric measurements of Δ14CO2 and the dual-tracer Δ14CO2:CO2 assimilation and inversion system previously developed by our group to estimate annual and monthly CO2 emissions from fossil fuel use and cement production (FFCO2) for the U.S. for 2010 and 2015, the first two individual years for which large numbers of atmospheric Δ14CO2 measurements are available. Ensemble-mean national FFCO2 totals obtained from a 9-member suite of inverse results are larger than reported by the U.S. Environmental Protection Agency (EPA), but overlap at their respective 2σ ensemble-wide model spreads (inversions) and reported 95 % confidence intervals (EPA) in both years. In contrast, the inverse results agree with both annual totals and 16 of 24 derived monthly totals from the Vulcan 3.0 emissions data product with 1σ, ensemble wide. Central estimates of the change in U.S. FFCO2 emission between 2010 and 2015 range from -5.1 % (EPA), -5.8 % (Vulcan), and -7.8 % (this work), providing a first confirmation of an expected national FFCO2 decline based on atmospheric observations. The development of a reliable emissions tracking system based directly on atmospheric observations, as detailed here, may take on additional scientific and policy relevance given the recent interruption of EPA reporting.

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S. M. Nazrul Islam, Scott J. Lehman, Sourish Basu, Arlyn E. Andrews, Kathryn McKain, Colm Sweeney, Xiaomei Xu, Chad Wolak, Stephen P. Morgan, Patrick Cappa, John R. Southon, Pieter P. Tans, and John B. Miller

Status: open (until 17 Aug 2026)

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S. M. Nazrul Islam, Scott J. Lehman, Sourish Basu, Arlyn E. Andrews, Kathryn McKain, Colm Sweeney, Xiaomei Xu, Chad Wolak, Stephen P. Morgan, Patrick Cappa, John R. Southon, Pieter P. Tans, and John B. Miller
S. M. Nazrul Islam, Scott J. Lehman, Sourish Basu, Arlyn E. Andrews, Kathryn McKain, Colm Sweeney, Xiaomei Xu, Chad Wolak, Stephen P. Morgan, Patrick Cappa, John R. Southon, Pieter P. Tans, and John B. Miller
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Latest update: 06 Jul 2026
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Short summary
This study uses carbon dioxide and atmospheric radiocarbon observations to estimate U.S. fossil fuel CO₂ emissions for 2010 and 2015. The results provide an independent atmospheric verification of national emission trends, showing a decline in FFCO₂ emissions and agreement with bottom-up inventories such as EPA and other estimates. The work highlights the value of atmospheric observations for greenhouse gas monitoring, emissions verification, and climate policy applications.
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