Preprints
https://doi.org/10.5194/egusphere-2025-4338
https://doi.org/10.5194/egusphere-2025-4338
14 Jan 2026
 | 14 Jan 2026
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Global transport of upper-tropospheric tropical tracers: multi-year insights from idealized simulations

Lianet Hernández Pardo, Joachim Curtius, Patrick Jöckel, Moritz Menken, and Anna Possner

Abstract. Recent studies suggest that significant aerosol formation occurs in the tropical upper troposphere (UT). However, the impact of these particles at lower levels remains poorly understood. We present results from multi-year global EMAC simulations investigating the downward transport of UT tracers and their resulting spatial distribution. Nineteen idealized tracers were released in the tropical UT and subjected to resolved-scale advection, parameterized convection, turbulent mixing, and wet/dry deposition. Transport timescales are highly sensitive to source extent: the age of air at 500 hPa is ≈45 days for tropical-wide tracers, compared to over 250 days for regional continental sources, reflecting the importance of mixing and dilution. A complementary time-to-threshold diagnostic reveals faster transport pathways, with all source regions exhibiting descent times shorter than 7 days to reach 10% of the source average. Advection dominates vertical transport, with convective and vertical diffusion parameterizations contributing marginally. Injection height exerts a stronger influence on descent time than parameterized transport or particle size in the 20100nm range. Tracer maxima are typically advected east of their source centers, resulting in significant concentrations (~1015% of source values) in the mid-troposphere. Offline calculations show that, for initial particle numbers below ~6×107 kg-1, the mid-troposphere values predicted by the model are reduced by less than 10% when coagulation is considered, but substantial deviations occur at higher concentrations. These results provide quantitative constraints on particle transport efficiency and inform expectations for aerosol distributions following UT nucleation events.

Competing interests: Two co-authors of the manuscript are topical editors of the journal.

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Lianet Hernández Pardo, Joachim Curtius, Patrick Jöckel, Moritz Menken, and Anna Possner

Status: open (until 25 Feb 2026)

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Lianet Hernández Pardo, Joachim Curtius, Patrick Jöckel, Moritz Menken, and Anna Possner
Lianet Hernández Pardo, Joachim Curtius, Patrick Jöckel, Moritz Menken, and Anna Possner

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Short summary
Many tiny particles are formed high in the tropical atmosphere, but their impact lower down is unclear. We studied how these particles move downward using long-term computer simulations. We found that particles can reach middle levels of the atmosphere within a week, carried by winds. These results help us understand how pollution and clouds might change as particles spread around the world.
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