Preprints
https://doi.org/10.5194/egusphere-2025-5998
https://doi.org/10.5194/egusphere-2025-5998
12 Dec 2025
 | 12 Dec 2025
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Anthropogenic Modulation of Dust-Dominated Ice Nucleation in an Urban Dryland City of China

Chengqing Chen, Yang Wang, Jiming Li, Lu Feng, Tianrong Chai, Zhao Ji, Jian Wang, and Yuan Wang

Abstract. Ice-nucleating particles (INPs) are crucial for cloud formation and precipitation, yet their variability and influencing factors in urban dryland regions remain poorly understood. While natural dust is recognized as the dominant INP source, the extent to which anthropogenic pollution modulates INP abundance remains insufficiently quantified. Here, we present online observations of INPs (−15 to −35 °C), together with co-located aerosol size distribution and chemical composition in Lanzhou from winter 2024 to spring 2025. We show that long-range dust transport boosts INP concentrations by × 15 at −30 °C. Elevated secondary inorganic aerosol during pollution was enhanced and negatively correlated with INP activity (R = −0.71). We further refine a two-parameter scheme (1–2.5 µm aerosol diameter and temperature) that reproduces 83 % of observations within a factor of 5. These findings underscore the need to include local aerosol heterogeneity and dust-pollution interactions in INPs parameterizations for more accurate regional climate simulations.

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Chengqing Chen, Yang Wang, Jiming Li, Lu Feng, Tianrong Chai, Zhao Ji, Jian Wang, and Yuan Wang

Status: open (until 23 Jan 2026)

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Chengqing Chen, Yang Wang, Jiming Li, Lu Feng, Tianrong Chai, Zhao Ji, Jian Wang, and Yuan Wang
Chengqing Chen, Yang Wang, Jiming Li, Lu Feng, Tianrong Chai, Zhao Ji, Jian Wang, and Yuan Wang
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Short summary
Our observations show that both local dust and dust carried over long distances can increase the number of particles that help form ice in clouds. Polluted air held fewer such particles and appears to weaken the ability of dust to initiate ice formation. In semi-arid cities, larger particles in the 1–2.5 µm range strongly indicate how many of these ice-forming particles are present. Understanding how different particles behave is essential for representing cloud glaciation and regional climate.
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