Preprints
https://doi.org/10.5194/egusphere-2025-3258
https://doi.org/10.5194/egusphere-2025-3258
17 Jul 2025
 | 17 Jul 2025

Emulating chemistry-climate dynamics with a linear inverse model

Eric John Mei, Gregory J. Hakim, Max Taniguchi-King, Dominik Stiller, and Alexander J. Turner

Abstract. Coupled chemistry–climate models (CCMs) are powerful tools for investigating chemical variability in the climate system, but high computational cost limits their use for hypothesis testing and adequately sampling variability on long timescales. Here, we present the first application of a linear inverse model (LIM) to emulate a CCM. A LIM is a lowdimensional empirical model that reproduces the CCM’s statistics and dynamics at low computational cost. By linearizing the CCM’s dynamics, the LIM captures coherent modes of variability, such as the El Niño Southern Oscillation (ENSO), that describe the coupled evolution of physical and chemical fields. Deterministic seasonal forecasts of the LIM result in skillful predictions of physical and chemical variables at lead times up to a year, outperforming damped persistence models. We show that the LIM’s skill in chemical fields depends on its coupled chemistry–climate modes: forecasts without the ENSO dynamical mode show a substantial loss of skill, suggesting the importance of ENSO in driving predictable chemical variability. These results demonstrate that the LIM can efficiently emulate CCM dynamics. It offers a practical tool for testing hypotheses about the drivers of chemistry-climate interactions and may enable efficient chemical data assimilation in the future.

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Eric John Mei, Gregory J. Hakim, Max Taniguchi-King, Dominik Stiller, and Alexander J. Turner

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  • RC1: 'Comment on egusphere-2025-3258', Anonymous Referee #1, 28 Aug 2025
  • RC2: 'Comment on egusphere-2025-3258', Anonymous Referee #2, 28 Aug 2025
Eric John Mei, Gregory J. Hakim, Max Taniguchi-King, Dominik Stiller, and Alexander J. Turner
Eric John Mei, Gregory J. Hakim, Max Taniguchi-King, Dominik Stiller, and Alexander J. Turner

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Short summary
Chemistry-climate models are used to investigate how physical climate influences the composition of the atmosphere but are slow and expensive to run. We train a linear inverse model that can replicate the behavior of chemistry-climate models at low computational cost. It captures how large-scale climate features like El Niño affect atmospheric composition and can make accurate forecasts up to a year ahead. This model enables fast hypothesis testing and estimates of past atmospheric composition.
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