Preprints
https://doi.org/10.5194/egusphere-2025-250
https://doi.org/10.5194/egusphere-2025-250
26 Mar 2025
 | 26 Mar 2025

Potential CO2 measurement capabilities of a transportable Near Infrared Laser Heterodyne Radiometer (LHR)

Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen

Abstract. Heterodyne detection stands as a powerful method for enhancing sensitivity limits and attaining exceptional resolution. It also offers the advantage of being transportable and the ability to make it more compact which makes it favorable for ground-based remote sensing in field campaigns. An all-fiber coupled laser heterodyne radiometer (LHR), using a wideband tunable external cavity diode laser (1520–1580 nm) as local oscillator laser was developed for CO2 measurements. Optimal absorption lines and transmission spectra of the LHR was achieved by using a balanced photodetector to suppress the relative intensity noise of the local oscillator laser. This work aims to quantify how the LHR contributes to measuring tropospheric CO2 abundances in the atmospheric column from the ground. Here, we demonstrate the LHR’s ability to measure CO2 vertical profiles through a extensive analysis of information content, channel selection, and error budget estimation. This comprehensive analysis relies on the radiative transfer model ARAHMIS, developed at the Laboratoire d’Optique Atmosphérique (LOA). Additionally, we present a comparison of the LHR with other ground-based instruments, such as the EM27/SUN and the IFS125HR from the TCCON network. Furthermore, this work supports ongoing MAGIC campaigns focused on greenhouse gas monitoring and the validation of current and future space missions such as MicroCarb and FORUM.

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Journal article(s) based on this preprint

12 Sep 2025
Potential CO2 measurement capabilities of a transportable Near Infrared Laser Heterodyne Radiometer (LHR)
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen
Atmos. Meas. Tech., 18, 4515–4526, https://doi.org/10.5194/amt-18-4515-2025,https://doi.org/10.5194/amt-18-4515-2025, 2025
Short summary
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2025-250', Anonymous Referee #1, 08 May 2025
  • EC1: 'Comment on egusphere-2025-250', Frank Hase, 26 May 2025
  • RC2: 'Comment on egusphere-2025-250', Anonymous Referee #2, 01 Jul 2025

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2025-250', Anonymous Referee #1, 08 May 2025
  • EC1: 'Comment on egusphere-2025-250', Frank Hase, 26 May 2025
  • RC2: 'Comment on egusphere-2025-250', Anonymous Referee #2, 01 Jul 2025

Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision | EF: Editorial file upload
AR by El Kattar Marie-Thérèse on behalf of the Authors (25 Jul 2025)  Author's response   Author's tracked changes   Manuscript 
EF by Daria Karpachova (29 Jul 2025)  Author's response 
EF by Daria Karpachova (29 Jul 2025)  Manuscript 
ED: Publish as is (29 Jul 2025) by Frank Hase
AR by El Kattar Marie-Thérèse on behalf of the Authors (29 Jul 2025)  Manuscript 

Journal article(s) based on this preprint

12 Sep 2025
Potential CO2 measurement capabilities of a transportable Near Infrared Laser Heterodyne Radiometer (LHR)
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen
Atmos. Meas. Tech., 18, 4515–4526, https://doi.org/10.5194/amt-18-4515-2025,https://doi.org/10.5194/amt-18-4515-2025, 2025
Short summary
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen

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The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.

Short summary
This study, part of my 2024 postdoctoral research at ULCO, explores an all-fiber coupled laser heterodyne radiometer (LHR) for CO2 measurements using a tunable diode laser. The LHR employs balanced detection to measure tropospheric CO2 column concentrations. Simulations with the ARAHMIS model are validated against instruments like EM27/SUN and IFS125HR. This work enhances greenhouse gas monitoring and supports campaigns like MAGIC for emissions studies and satellite validation.
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