Preprints
https://doi.org/10.5194/egusphere-2024-3586
https://doi.org/10.5194/egusphere-2024-3586
26 Nov 2024
 | 26 Nov 2024

Stratospheric Aerosol Intervention Experiment for the Chemistry-Climate Model Intercomparison Project

Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer

Abstract. A new Stratospheric Aerosol Intervention (SAI) experiment has been designed for the Chemistry- Climate Modeling Initiative (CCMI-2022) to assess the impacts of SAI on stratospheric chemistry and dynamical responses and inter-model differences using a constrained setup with a prescribed stratospheric aerosol distribution and fixed sea-surface temperatures (SSTs) and sea-ice. This paper describes the details of the experimental setup and the prescribed aerosol distribution. Furthermore, we discuss differences in the Whole Atmosphere Community Climate Model (WACCM6) results between the interactive stratospheric aerosol configuration with coupling to land, ocean, and sea ice that was used to produce the stratospheric aerosol distribution and the results of the constrained SAI experiment. With this, we identify and isolate the stratosphere-controlled SAI-induced impacts from those influenced by the coupling with the ocean. We confirm earlier suggestions that the SAI-induced positive phase of the Northern Atlantic Oscillation in winter, with the corresponding winter warming over Eurasia, is directly driven by the effect of SAI on the stratosphere-troposphere coupling. We further show that the resulting stratospheric responses are largely similar between the fully coupled and constrained experiments, demonstrating the suitability of the simplified setup to study impacts in the stratosphere in a multi-model framework. Only small differences arise in the stratospheric ozone and dynamical SAI responses between the two experiments due to minor differences in the aerosol distributions and their coupling with local changes in temperatures, upwelling, and chemistry, alongside interactive coupling with the ocean and sea ice.

Competing interests: ST and EMB are members of the editorial board of the journal.

Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this preprint. The responsibility to include appropriate place names lies with the authors.
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Journal article(s) based on this preprint

18 Jun 2025
Stratospheric Aerosol Intervention experiment for the Chemistry–Climate Model Initiative
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
Atmos. Chem. Phys., 25, 6001–6023, https://doi.org/10.5194/acp-25-6001-2025,https://doi.org/10.5194/acp-25-6001-2025, 2025
Short summary
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2024-3586', Anonymous Referee #1, 11 Dec 2024
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025
  • RC2: 'Comment on egusphere-2024-3586', Anonymous Referee #2, 27 Dec 2024
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025
  • RC3: 'Comment on egusphere-2024-3586', Anonymous Referee #3, 07 Jan 2025
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2024-3586', Anonymous Referee #1, 11 Dec 2024
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025
  • RC2: 'Comment on egusphere-2024-3586', Anonymous Referee #2, 27 Dec 2024
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025
  • RC3: 'Comment on egusphere-2024-3586', Anonymous Referee #3, 07 Jan 2025
    • AC1: 'Reply on RC2', Simone Tilmes, 17 Feb 2025

Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision | EF: Editorial file upload
AR by Simone Tilmes on behalf of the Authors (17 Feb 2025)  Author's response   Author's tracked changes   Manuscript 
ED: Publish subject to minor revisions (review by editor) (25 Feb 2025) by Petr Šácha
AR by Simone Tilmes on behalf of the Authors (04 Mar 2025)  Author's response   Author's tracked changes   Manuscript 
ED: Publish as is (05 Mar 2025) by Petr Šácha
AR by Simone Tilmes on behalf of the Authors (14 Mar 2025)

Journal article(s) based on this preprint

18 Jun 2025
Stratospheric Aerosol Intervention experiment for the Chemistry–Climate Model Initiative
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
Atmos. Chem. Phys., 25, 6001–6023, https://doi.org/10.5194/acp-25-6001-2025,https://doi.org/10.5194/acp-25-6001-2025, 2025
Short summary
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer

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Short summary
This paper describes the details of a new multi-model intercomparison experiment to assess the effects of Stratospheric Aerosol Injections on stratospheric chemistry and dynamics and, therefore, ozone. In this experiment, all models will use the same prescribed stratospheric aerosol distribution and fixed sea-surface temperatures and sea ice. We discuss the advantages and differences of this more constrained experiment compared to previous more interactive model experiments.
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