Preprints
https://doi.org/10.5194/egusphere-2024-3057
https://doi.org/10.5194/egusphere-2024-3057
23 Oct 2024
 | 23 Oct 2024
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Strong inter-model differences and biases in CMIP6 simulations of PM2.5, aerosol optical depth, and precipitation over Africa

Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt

Abstract. Poor air quality and precipitation change are strong, rapidly changing, and possibly linked, drivers of physical hazards in sub-Saharan Africa. Future projections of sub-Saharan air quality and precipitation remain uncertain due to differences in model representations of aerosol, aerosol-precipitation interactions, and unclear future aerosol emission pathways. In this study, we evaluate the performance of CMIP6 models in simulating PM2.5, aerosol optical depth (AOD), and precipitation over Africa, relative to a range of observational and reanalysis products, including novel observational datasets, over the 1981–2023 period. While models accurately capture the seasonal cycle of PM2.5 concentrations over most regions, the concentration magnitudes show strong inter-model diversity. Dust AOD shows generally accurate seasonal spatial distribution, with multi-model mean (MMM) pattern correlation coefficients within 0.77–0.94, despite strong inter-model diversity in magnitude. Seasonal spatial patterns of non-dust AOD are poorly represented, with MMM pattern correlation coefficients of 0.25–0.58, and poorest performance during SON. Emission inventory inaccuracies may explain systematic biases for non-dust AOD fields, with differences in circulation and precipitation patterns, and aerosol treatment causing inter-model diversity. Both monsoon regions are generally well captured, though there is poorer performance in simulating the east African monsoon. Biases found relate to the intertropical convergence zone, more apparent over east Africa, and rainfall magnitude, more apparent over west Africa. This evaluation highlights strong inter-model diversity in the representation of African air quality and climate, and identifies model performance over sub-Saharan Africa, and the reasons behind the biases, as critical gaps to address for improving confidence in climate projections.

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Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt

Status: open (until 04 Dec 2024)

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Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt

Data sets

CHIRPS: Rainfall Estimates from Rain Gauge and Satellite Observations C. C. Funk et al. https://doi.org/10.1038/sdata.2015.66

The Earth System Grid Federation: An open infrastructure for access to distributed geospatial data L. Cinquini et al. https://doi.org/10.1016/j.future.2013.07.002

ECMWF Reanalysis v5 (ERA5) H. Hersbach et al. https://www.ecmwf.int/en/forecasts/dataset/ecmwf-reanalysis-v5

CAMS global reanalysis (EAC4) A. Inness et al. https://doi.org/10.5194/acp-19-3515-2019

Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt

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Short summary
Our research explores how well air pollution and rainfall patterns in Africa are represented in current climate models, by comparing model data to observations from 1981 to 2023. While most models capture seasonal air quality changes well, they struggle to replicate the distribution of non-dust pollutants and certain rainfall patterns, especially over east Africa. Improving these models is crucial for better climate predictions and preparing for future risks.