Preprints
https://doi.org/10.5194/egusphere-2024-2764
https://doi.org/10.5194/egusphere-2024-2764
18 Sep 2024
 | 18 Sep 2024
Status: this preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).

Robustness of atmospheric trace gas retrievals obtained from low spectral resolution Fourier-transform infrared absorption spectra

Bavo Langerock, Martine De Mazière, Filip Desmet, Pauli Heikkinen, Rigel Kivi, Mahesh Kumar Sha, Corinne Vigouroux, Minqiang Zhou, Gopala Khrisna Darbha, and Mohmmed Talib

Abstract. For atmospheric trace gas columns retrievals obtained from ground based Fourier-transform interferometer spectra we study the sensitivity of the retrieval processing chain to changes in the number of points in the recorded interferograms. Shortening an interferogram will alter the leakage pattern in the associated spectrum and we demonstrate that the removal of a relatively small number of points from the interferogram edges creates a beat pattern in the difference of the associated spectra obtained from the original and shortened interferogram. For low-resolution interferometers the beat pattern in the spectra may exceed the noise level and the effect on atmospheric gas column retrievals may be large. Sensitivity of the retrieval algorithm to the length of the underlying interferogram can be reduced by applying a non-trivial apodization such as Norton-Beer. A case study shows the effect on formaldehyde retrievals obtained from low-resolution spectra in Sodankylä and Kolkata.

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Bavo Langerock, Martine De Mazière, Filip Desmet, Pauli Heikkinen, Rigel Kivi, Mahesh Kumar Sha, Corinne Vigouroux, Minqiang Zhou, Gopala Khrisna Darbha, and Mohmmed Talib

Status: open (until 31 Oct 2024)

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Bavo Langerock, Martine De Mazière, Filip Desmet, Pauli Heikkinen, Rigel Kivi, Mahesh Kumar Sha, Corinne Vigouroux, Minqiang Zhou, Gopala Khrisna Darbha, and Mohmmed Talib
Bavo Langerock, Martine De Mazière, Filip Desmet, Pauli Heikkinen, Rigel Kivi, Mahesh Kumar Sha, Corinne Vigouroux, Minqiang Zhou, Gopala Khrisna Darbha, and Mohmmed Talib

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Short summary
Ground-based Fourier-transform interferometer instruments have been used for many decades to measure direct solar light in the infrared to obtain high-resolution spectra from which atmospheric gas profile concentrations can be derived. It is shown that the typical processing chain used to derive atmospheric gas columns can be sensitive to relatively small shortenings of the recorded interferograms. Low-resolution recordings, used in more recent years, are more sensitive to such adaptations.