Preprints
https://doi.org/10.5194/egusphere-2024-2736
https://doi.org/10.5194/egusphere-2024-2736
20 Sep 2024
 | 20 Sep 2024
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Large Reductions in Satellite-Derived and Modelled European Lower Tropospheric Ozone During and After the COVID-19 Pandemic (2020–2022)

Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Wuhu Feng, and Martyn P. Chipperfield

Abstract. Activity restrictions during the COVID-19 pandemic caused large reductions in ozone (O3) precursor emissions. Studies showed large O3 reductions in the 2020 spring-summer Northern Hemisphere free troposphere coinciding with this emission reduction period. Here, we provide an insight into the European satellite-derived tropospheric O3 record updated to mid-2023. Rutherford Appleton Laboratory (RAL) retrieval products show large negative anomalies in the spring-summer periods of 2020–2022, with the largest in 2022, and smaller reductions in 2023. The Infrared Atmospheric Sounding Interferometer (IASI) showed peak reductions compared to monthly averages of 2.2 DU (11.0 %), 1.7 DU (8.4 %) and 2.8 DU (14.6 %) in 2020, 2021 and 2022, respectively. Scaling model emissions, based on activity reduction data, yields large negative anomalies peaking in May 2020 and 2021. Emissions reduction was the greater influence, explaining ~65 % of the decrease, however, the meteorological impact was substantial, driven by a reduced stratosphere-troposphere O3 exchange flux.

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Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Wuhu Feng, and Martyn P. Chipperfield

Status: open (until 01 Nov 2024)

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Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Wuhu Feng, and Martyn P. Chipperfield
Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Wuhu Feng, and Martyn P. Chipperfield

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Short summary
Globally, lockdowns were implemented to limit the spread of COVID-19, leading to a decrease in emissions of key air pollutants. Here, we use novel satellite data and a chemistry model to investigate the impact of the pandemic on tropospheric ozone (O3), a key pollutant, in 2020. Overall, we found substantial decreases of up to 20 %, 2/3s of which came from emission reductions while 1/3 was due to a decrease in the stratospheric ozone flux into the troposphere.