Preprints
https://doi.org/10.5194/egusphere-2024-2457
https://doi.org/10.5194/egusphere-2024-2457
26 Aug 2024
 | 26 Aug 2024
Status: this preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).

Multi-observational estimation of regional and sectoral emission contributions to the persistent high growth rate of atmospheric CH4 for 2020–2022

Yosuke Niwa, Yasunori Tohjima, Yukio Terao, Tazu Saeki, Akihiko Ito, Taku Umezawa, Kyohei Yamada, Motoki Sasakawa, Toshinobu Machida, Shin-Ichiro Nakaoka, Hideki Nara, Hiroshi Tanimoto, Hitoshi Mukai, Yukio Yoshida, Shinji Morimoto, Shinya Takatsuji, Kazuhiro Tsuboi, Yousuke Sawa, Hidekazu Matsueda, Kentaro Ishijima, Ryo Fujita, Daisuke Goto, Xin Lan, Kenneth Schuldt, Michal Heliasz, Tobias Biermann, Lukasz Chmura, Jarsolaw Necki, and Irène Xueref-Remy

Abstract. An inverse study of atmospheric methane (CH4) estimated regional and sectoral emission contributions to the unprecedented surge of the atmospheric growth rate for 2020–2022. Three inverse analyses, which used only surface observations, surface and aircraft observations, and satellite (GOSAT) observations, consistently suggested notable emission increases in the tropics (15° S–10° N) (10–18 Tg CH4 yr−1) and in northern low-latitudes (10–35° N) (ca. 20 Tg CH4 yr−1), the latter of which likely contributed to the growth rate surge from 2020. The emission increase in the northern low-latitudes is attributed to emissions in South Asia (6–7 Tg CH4 yr−1) and northern Southeast Asia (5 Tg CH4 yr−1), which abruptly increased from 2019 to 2020, and elevated emissions continued until 2022. Meanwhile, the tropical emission increase is dominated by tropical South America (5–7 Tg CH4 yr−1) and central Africa (3–6 Tg CH4 yr−1), but they were continuously increasing before 2019. Agreement was found in sectoral estimates in the tropics and northern low-latitudes, suggesting that biogenic emissions from wetlands, agriculture, and waste are the largest contributors. High-precision surface and aircraft observations imposed constraints that were comparable to or 1.5 times stronger than GOSAT constraints on the flux estimates in South and Southeast Asia. Furthermore, a sensitivity inversion test suggested that the effect of the probable reduction of OH radicals in 2020 might be limited in the Asian regions. These results highlight the importance of biogenic emissions in Asian regions for the persistent high growth rate observed during 2020–2022.

Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this preprint. The responsibility to include appropriate place names lies with the authors.
Yosuke Niwa, Yasunori Tohjima, Yukio Terao, Tazu Saeki, Akihiko Ito, Taku Umezawa, Kyohei Yamada, Motoki Sasakawa, Toshinobu Machida, Shin-Ichiro Nakaoka, Hideki Nara, Hiroshi Tanimoto, Hitoshi Mukai, Yukio Yoshida, Shinji Morimoto, Shinya Takatsuji, Kazuhiro Tsuboi, Yousuke Sawa, Hidekazu Matsueda, Kentaro Ishijima, Ryo Fujita, Daisuke Goto, Xin Lan, Kenneth Schuldt, Michal Heliasz, Tobias Biermann, Lukasz Chmura, Jarsolaw Necki, and Irène Xueref-Remy

Status: open (extended)

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  • RC1: 'Comment on egusphere-2024-2457', Anonymous Referee #1, 22 Oct 2024 reply
Yosuke Niwa, Yasunori Tohjima, Yukio Terao, Tazu Saeki, Akihiko Ito, Taku Umezawa, Kyohei Yamada, Motoki Sasakawa, Toshinobu Machida, Shin-Ichiro Nakaoka, Hideki Nara, Hiroshi Tanimoto, Hitoshi Mukai, Yukio Yoshida, Shinji Morimoto, Shinya Takatsuji, Kazuhiro Tsuboi, Yousuke Sawa, Hidekazu Matsueda, Kentaro Ishijima, Ryo Fujita, Daisuke Goto, Xin Lan, Kenneth Schuldt, Michal Heliasz, Tobias Biermann, Lukasz Chmura, Jarsolaw Necki, and Irène Xueref-Remy
Yosuke Niwa, Yasunori Tohjima, Yukio Terao, Tazu Saeki, Akihiko Ito, Taku Umezawa, Kyohei Yamada, Motoki Sasakawa, Toshinobu Machida, Shin-Ichiro Nakaoka, Hideki Nara, Hiroshi Tanimoto, Hitoshi Mukai, Yukio Yoshida, Shinji Morimoto, Shinya Takatsuji, Kazuhiro Tsuboi, Yousuke Sawa, Hidekazu Matsueda, Kentaro Ishijima, Ryo Fujita, Daisuke Goto, Xin Lan, Kenneth Schuldt, Michal Heliasz, Tobias Biermann, Lukasz Chmura, Jarsolaw Necki, and Irène Xueref-Remy

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Short summary
This study estimated regional and sectoral emission contributions to the unprecedented surge of atmospheric methane for 2020–2022. The methane is the second most important greenhouse gas and its emissions reduction is urgently required to mitigate the global warming. Numerical modeling-based estimates with three different sets of atmospheric observations consistently suggested large contributions of biogenic emissions from South Asia and Southeast Asia to the surge of atmospheric methane.