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Preprints
https://doi.org/10.5194/egusphere-2024-1887
https://doi.org/10.5194/egusphere-2024-1887
28 Jun 2024
 | 28 Jun 2024

Age of air from in situ trace gas measurements: Insights from a new technique

Eric A. Ray, Fred L. Moore, Hella Garny, Eric J. Hintsa, Bradley D. Hall, Geoff S. Dutton, David Nance, James W. Elkins, Steven C. Wofsy, Jasna Pittman, Bruce Daube, Bianca C. Baier, Jianghanyang Li, and Colm Sweeney

Abstract. The age of air is an important transport diagnostic that can be derived from trace gas measurements and compared to global chemistry climate model output.  We describe a new technique to calculate the age of air, measuring transport times from the Earth’s surface to any location in the atmosphere based on simultaneous in situ measurements of multiple key long-lived trace gases. The primary benefits of this new technique include (1) optimized ages of air consistent with simultaneously measured SF6 and CO2, (2) age of air from the upper troposphere through the stratosphere, (3) estimates of the second moment of age spectra that have not been well constrained from measurements and (4) flexibility to be used with measurements across multiple instruments, platforms and decades.  We demonstrate the technique on aircraft and balloon measurements from the 1990s, the last period of extensive stratospheric in situ sampling, and several recent missions from the 2020s, and compare the results with previously published and modeled values.

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Journal article(s) based on this preprint

11 Nov 2024
Age of air from in situ trace gas measurements: insights from a new technique
Eric A. Ray, Fred L. Moore, Hella Garny, Eric J. Hintsa, Bradley D. Hall, Geoff S. Dutton, David Nance, James W. Elkins, Steven C. Wofsy, Jasna Pittman, Bruce Daube, Bianca C. Baier, Jianghanyang Li, and Colm Sweeney
Atmos. Chem. Phys., 24, 12425–12445, https://doi.org/10.5194/acp-24-12425-2024,https://doi.org/10.5194/acp-24-12425-2024, 2024
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In this study we describe new techniques to derive age of air from multiple simultaneous...
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