the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
| 17 Jun 2024
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK climate model
Abstract. Changes in the availability of a subset of aerosol known as ice-nucleating particles (INPs) can substantially alter cloud microphysical and radiative properties. Despite very large spatial and temporal variability in INP properties, many climate models do not currently represent the link between the global distribution of aerosols and INPs, and primary ice production in clouds. Here we use the UK Earth System Model to simulate the global distribution of dust and marine-sourced INPs over an annual cycle. The model captures the overall spatial and temporal distribution of measured INP concentrations, which is strongly influenced by the world’s major mineral dust source regions. A negative bias in simulated versus measured INP concentrations at higher freezing temperatures points to incorrectly defined INP properties or a missing source of INPs. We find that the ability of the model to reproduce measured INP concentrations is greatly improved by representing dust as a mixture of mineralogical and organic ice-nucleating components, as present in many soils. To improve the agreement further, we define an optimized hypothetical parameterization of dust INP activity (ns(T)) as a function of temperature with a logarithmic slope of -0.175 K−1, which is much shallower than existing parameterizations (e.g., -0.35 K−1 for the K-feldspar data of Harrison et al. (2019)). The results point to a globally important role for an organic component associated with mineral dust.
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Notice on discussion status
The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.
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Preprint
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Supplement
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The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.
- Preprint
(15152 KB) - Metadata XML
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Supplement
(1351 KB) - BibTeX
- EndNote
- Final revised paper
Journal article(s) based on this preprint
Interactive discussion
Status: closed
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RC1: 'Comment on egusphere-2024-1538', Anonymous Referee #1, 07 Jul 2024
General comments:
In this paper, the authors present a comprehensive study on simulating the global distribution of dust and marine ice-nucleating particles (INPs) using the UK Earth System Model (UKESM1). They incorporate two important INP types, namely dust and marine organic aerosols, into the model and evaluate the simulations against an expanded global dataset of INP measurements. Furthermore, they found that soil dust might be an important INP source which was not considered in the current model. The paper is well-structured and clearly written. The methodology is sound, and the results are presented in a logical and convincing manner. The study makes a significant contribution to understanding the global distribution of INPs and identifying potential gaps in current INP representations in climate models. The paper is a valuable contribution to the field and provides useful insights into the gaps in our understanding of INP sources and their representation in climate models. I recommend publication after addressing the following comments:
Model evaluation using satellite observations:
The authors demonstrate the model's skill in capturing the spatial and temporal variability of INP concentrations through a thorough comparison with observations from diverse geographical locations and seasons. However, as the authors acknowledge, the current INP observations are primarily short-term campaign measurements, lacking long-term continuous time series. Relying solely on these ground-based INP observations may not be sufficient for a comprehensive evaluation of the model's performance. To address this limitation, I suggest that the authors consider utilizing satellite remote sensing data to further validate their model results. Satellites can provide valuable information on cloud phase and cloud-top temperature, which can be used to infer the threshold temperature for immersion freezing INPs (Carlsen et al., 2022). This satellite-based diagnostic approach can help identify potential INP sources on a global scale, complementing the ground-based observations. The authors should discuss the advantages and limitations of using satellite data for model validation in their discussion section.
Potential role of anthropogenic pollution in the Northern Hemisphere mid to high latitudes:
The most intriguing finding of this study is the discrepancy between the observed and modeled ice-nucleating particle (INP) concentrations in the mid to high latitudes of the Northern Hemisphere, particularly at higher temperatures. The authors suggest that soil dust may be an overlooked source of INPs in these regions. This insight opens up a new avenue for investigation and highlights the need to better understand the role of different INP sources in the global context. However, it is important to note that the mid to high latitudes of the Northern Hemisphere are also heavily influenced by anthropogenic pollution. While the contribution of anthropogenic pollutants to INP concentrations is still a matter of ongoing research and debate, there is evidence from satellite observations and field measurements that cannot be ignored. Satellite-based studies have shown that polluted regions tend to exhibit higher ice nucleation threshold temperatures, indicating a potential impact of anthropogenic emissions on ice formation processes (Zhao et al., 2019). Additionally, some recent observation found that organic aerosols in anthropogenically influenced areas can importantly contribute to INP concentrations (Tian et al., 2022). These studies should be referenced for more comprehensive explanations of your results.
Given these findings, I suggest that the authors consider the potential role of anthropogenic pollution in their analysis and discussion. While soil dust may indeed be an important and overlooked source of INPs, the influence of anthropogenic pollutants should not be dismissed, especially in regions where their concentrations are high. The authors could strengthen their argument by addressing this aspect and discussing how the relative contributions of soil dust and anthropogenic pollutants to INP concentrations might vary spatially and temporally. By considering the potential role of anthropogenic pollution alongside soil dust, the authors can provide a more comprehensive analysis of the factors contributing to the observed discrepancies in INP concentrations in the Northern Hemisphere mid to high latitudes.
Reference:
Carlsen, T., & David, R. O. (2022). Spaceborne evidence that ice-nucleating particles influence high-latitude cloud phase. Geophysical Research Letters, 49, e2022GL098041. https://doi.org/10.1029/2022GL098041.
Zhao, B., Wang, Y., Gu, Y. et al. Ice nucleation by aerosols from anthropogenic pollution. Nat. Geosci. 12, 602–607 (2019). https://doi.org/10.1038/s41561-019-0389-4
Tian, P., Liu, D., Bi, K., Huang, M., Wu, Y., Hu, K., et al. (2022). Evidence for anthropogenic organic aerosols contributing to ice nucleation. Geophysical Research Letters, 49, e2022GL099990. https://doi.org/10.1029/2022GL099990
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RC2: 'Comment on egusphere-2024-1538', Anonymous Referee #2, 31 Aug 2024
The comment was uploaded in the form of a supplement: https://egusphere.copernicus.org/preprints/2024/egusphere-2024-1538/egusphere-2024-1538-RC2-supplement.pdf
- AC1: 'Response to referees', Ross Herbert, 07 Oct 2024
Interactive discussion
Status: closed
-
RC1: 'Comment on egusphere-2024-1538', Anonymous Referee #1, 07 Jul 2024
General comments:
In this paper, the authors present a comprehensive study on simulating the global distribution of dust and marine ice-nucleating particles (INPs) using the UK Earth System Model (UKESM1). They incorporate two important INP types, namely dust and marine organic aerosols, into the model and evaluate the simulations against an expanded global dataset of INP measurements. Furthermore, they found that soil dust might be an important INP source which was not considered in the current model. The paper is well-structured and clearly written. The methodology is sound, and the results are presented in a logical and convincing manner. The study makes a significant contribution to understanding the global distribution of INPs and identifying potential gaps in current INP representations in climate models. The paper is a valuable contribution to the field and provides useful insights into the gaps in our understanding of INP sources and their representation in climate models. I recommend publication after addressing the following comments:
Model evaluation using satellite observations:
The authors demonstrate the model's skill in capturing the spatial and temporal variability of INP concentrations through a thorough comparison with observations from diverse geographical locations and seasons. However, as the authors acknowledge, the current INP observations are primarily short-term campaign measurements, lacking long-term continuous time series. Relying solely on these ground-based INP observations may not be sufficient for a comprehensive evaluation of the model's performance. To address this limitation, I suggest that the authors consider utilizing satellite remote sensing data to further validate their model results. Satellites can provide valuable information on cloud phase and cloud-top temperature, which can be used to infer the threshold temperature for immersion freezing INPs (Carlsen et al., 2022). This satellite-based diagnostic approach can help identify potential INP sources on a global scale, complementing the ground-based observations. The authors should discuss the advantages and limitations of using satellite data for model validation in their discussion section.
Potential role of anthropogenic pollution in the Northern Hemisphere mid to high latitudes:
The most intriguing finding of this study is the discrepancy between the observed and modeled ice-nucleating particle (INP) concentrations in the mid to high latitudes of the Northern Hemisphere, particularly at higher temperatures. The authors suggest that soil dust may be an overlooked source of INPs in these regions. This insight opens up a new avenue for investigation and highlights the need to better understand the role of different INP sources in the global context. However, it is important to note that the mid to high latitudes of the Northern Hemisphere are also heavily influenced by anthropogenic pollution. While the contribution of anthropogenic pollutants to INP concentrations is still a matter of ongoing research and debate, there is evidence from satellite observations and field measurements that cannot be ignored. Satellite-based studies have shown that polluted regions tend to exhibit higher ice nucleation threshold temperatures, indicating a potential impact of anthropogenic emissions on ice formation processes (Zhao et al., 2019). Additionally, some recent observation found that organic aerosols in anthropogenically influenced areas can importantly contribute to INP concentrations (Tian et al., 2022). These studies should be referenced for more comprehensive explanations of your results.
Given these findings, I suggest that the authors consider the potential role of anthropogenic pollution in their analysis and discussion. While soil dust may indeed be an important and overlooked source of INPs, the influence of anthropogenic pollutants should not be dismissed, especially in regions where their concentrations are high. The authors could strengthen their argument by addressing this aspect and discussing how the relative contributions of soil dust and anthropogenic pollutants to INP concentrations might vary spatially and temporally. By considering the potential role of anthropogenic pollution alongside soil dust, the authors can provide a more comprehensive analysis of the factors contributing to the observed discrepancies in INP concentrations in the Northern Hemisphere mid to high latitudes.
Reference:
Carlsen, T., & David, R. O. (2022). Spaceborne evidence that ice-nucleating particles influence high-latitude cloud phase. Geophysical Research Letters, 49, e2022GL098041. https://doi.org/10.1029/2022GL098041.
Zhao, B., Wang, Y., Gu, Y. et al. Ice nucleation by aerosols from anthropogenic pollution. Nat. Geosci. 12, 602–607 (2019). https://doi.org/10.1038/s41561-019-0389-4
Tian, P., Liu, D., Bi, K., Huang, M., Wu, Y., Hu, K., et al. (2022). Evidence for anthropogenic organic aerosols contributing to ice nucleation. Geophysical Research Letters, 49, e2022GL099990. https://doi.org/10.1029/2022GL099990
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RC2: 'Comment on egusphere-2024-1538', Anonymous Referee #2, 31 Aug 2024
The comment was uploaded in the form of a supplement: https://egusphere.copernicus.org/preprints/2024/egusphere-2024-1538/egusphere-2024-1538-RC2-supplement.pdf
- AC1: 'Response to referees', Ross Herbert, 07 Oct 2024
Peer review completion
Journal article(s) based on this preprint
Data sets
Dataset for manuscript "Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK climate model" Ross J. Herbert https://doi.org/10.5281/zenodo.11186250
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Alberto Sanchez-Marroquin
Daniel P. Grosvenor
Kirsty J. Pringle
Stephen R. Arnold
Benjamin J. Murray
Kenneth S. Carslaw
The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.
- Preprint
(15152 KB) - Metadata XML
-
Supplement
(1351 KB) - BibTeX
- EndNote
- Final revised paper