Preprints
https://doi.org/10.5194/egusphere-2023-813
https://doi.org/10.5194/egusphere-2023-813
16 May 2023
 | 16 May 2023

Rapid saturation of cloud water adjustments to shipping emissions

Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier

Abstract. Human aerosol emissions change cloud properties by providing additional cloud condensation nuclei. This increases cloud droplet numbers, which in turn affects other cloud properties like liquid water content, and ultimately cloud albedo. These adjustments are poorly constrained, making aerosol effects the most uncertain part of anthropogenic climate forcing. Here we show that cloud droplet number and water content react differently to changing emission amounts in shipping exhausts. We use information about ship positions and modelled emission amounts together with reanalysis winds and satellite retrievals of cloud properties. The analysis reveals that cloud droplet numbers respond linearly to emission amount over a large range (1–10 kg h−1), before the response saturates. Liquid water increases in raining clouds, and increases are constant over the emission ranges observed. There is evidence that this is due to compensating effects under rainy and non-rainy conditions, consistent with suppression of rain by enhanced aerosol. This has implications for our understanding of cloud processes and may improve the way clouds are represented in climate models, in particular by changing parameterizations of liquid water responses to aerosol.

Journal article(s) based on this preprint

09 Oct 2023
| ACP Letters
| Highlight paper
Rapid saturation of cloud water adjustments to shipping emissions
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023,https://doi.org/10.5194/acp-23-12545-2023, 2023
Short summary Executive editor

Peter Manshausen et al.

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2023-813', Anonymous Referee #1, 29 May 2023
  • RC2: 'Comment on egusphere-2023-813', Anonymous Referee #2, 16 Jun 2023
  • AC1: 'Comment on egusphere-2023-813', Peter Manshausen, 19 Jul 2023

Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2023-813', Anonymous Referee #1, 29 May 2023
  • RC2: 'Comment on egusphere-2023-813', Anonymous Referee #2, 16 Jun 2023
  • AC1: 'Comment on egusphere-2023-813', Peter Manshausen, 19 Jul 2023

Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision | EF: Editorial file upload
AR by Peter Manshausen on behalf of the Authors (19 Jul 2023)  Author's response   Manuscript 
EF by Lorena Grabowski (20 Jul 2023)  Author's tracked changes 
ED: Referee Nomination & Report Request started (28 Jul 2023) by Martina Krämer
RR by Anonymous Referee #1 (29 Jul 2023)
RR by Anonymous Referee #2 (31 Jul 2023)
ED: Publish subject to technical corrections (15 Aug 2023) by Martina Krämer
ED: Publish as is (18 Aug 2023) by Timothy Garrett (Executive editor)
AR by Peter Manshausen on behalf of the Authors (01 Sep 2023)  Manuscript 

Journal article(s) based on this preprint

09 Oct 2023
| ACP Letters
| Highlight paper
Rapid saturation of cloud water adjustments to shipping emissions
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023,https://doi.org/10.5194/acp-23-12545-2023, 2023
Short summary Executive editor

Peter Manshausen et al.

Peter Manshausen et al.

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The requested preprint has a corresponding peer-reviewed final revised paper. You are encouraged to refer to the final revised version.

Ship tracks are enhanced regions of cloud brightness that trail behind ships that are known to be created by their effluent. They are widely used as observational test beds to deepen understanding of how pollution might affect cloud microphysical processes and climate at larger regional and global scales.  This study uses satellite observations of cloud properties and records of ship position and their effluent to assess perturbations from ship emissions on cloud droplet number and liquid water path. The study found that, as expected, the droplet number perturbation in shiptracks scales with ship emission rates of aerosol particles. Surprisingly, however, the liquid water path in drizzling clouds increased by an amount that was nearly fixed. The observation points to novel non-linear threshold behaviours of relevance to representations of aerosol indirect effects in climate models.
Short summary
Aerosol from burning fuel changes cloud properties, e.g. the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.