Preprints
https://doi.org/10.5194/egusphere-2023-1431
https://doi.org/10.5194/egusphere-2023-1431
25 Jul 2023
 | 25 Jul 2023

Interannual variability of summertime formaldehyde (HCHO) vertical column density and its main drivers in northern high latitudes

Tianlang Zhao, Jingqiu Mao, Zolal Ayazpour, Gonzalo González Abad, Caroline Nowlan, and Yiqi Zheng

Abstract. The northern high latitudes (50–90° N, mostly including boreal forest and tundra ecosystem) has been undergoing rapid climate and ecological changes over recent decades, leading to significant variations in volatile organic compounds (VOCs) emissions from biogenic and biomass burning sources. HCHO, a widely used indicator of VOC emission, exhibits high climate sensitivity. However, the interannual variability of HCHO and its main drivers over the region remain unclear. In this study, we use the GEOS-Chem chemical transport model and satellite retrievals from Ozone Monitoring Instrument (OMI) and Ozone Mapping and Profiler Suite (OMPS) to examine HCHO vertical column density (VCD) interannual variations in summertime of 2005–2019. Our results show that wildfires heavily influence interannual variability of HCHO VCD over Siberia, Alaska, and North Canada, while biogenic emissions and background methane oxidation are the predominant drivers of HCHO interannual variability over East Europe. Solar-induced chlorophyll fluorescence (SIF) from Orbiting Carbon Observatory-2 (OCO-2) provides additional evaluation for HCHO interannual variability from biogenic emission, showing potential of constraining biogenic emission in northern high latitudes.

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Tianlang Zhao, Jingqiu Mao, Zolal Ayazpour, Gonzalo González Abad, Caroline Nowlan, and Yiqi Zheng

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2023-1431', Anonymous Referee #1, 01 Sep 2023
    • AC2: 'Reply on RC1', Tianlang Zhao, 05 Feb 2024
  • RC2: 'Comment on egusphere-2023-1431', Anonymous Referee #2, 10 Oct 2023
    • AC1: 'Reply on RC2', Tianlang Zhao, 05 Feb 2024

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2023-1431', Anonymous Referee #1, 01 Sep 2023
    • AC2: 'Reply on RC1', Tianlang Zhao, 05 Feb 2024
  • RC2: 'Comment on egusphere-2023-1431', Anonymous Referee #2, 10 Oct 2023
    • AC1: 'Reply on RC2', Tianlang Zhao, 05 Feb 2024
Tianlang Zhao, Jingqiu Mao, Zolal Ayazpour, Gonzalo González Abad, Caroline Nowlan, and Yiqi Zheng
Tianlang Zhao, Jingqiu Mao, Zolal Ayazpour, Gonzalo González Abad, Caroline Nowlan, and Yiqi Zheng

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Short summary
This work aims at investigate the role of background HCHO, biogenic and wildfire emission in HCHO interannual variability over northern high latitudes. This work highlights the predominant role of wildfire in northern high latitudes during fire seasons, based on satellite HCHO, solar induced fluorescence (SIF) retrievals and GEOS-Chem model. The coupling between satellite SIF and biogenic emission over northern high latitudes shows the potential of SIF to constrain biogenic HCHO in this region.