<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "https://jats.nlm.nih.gov/nlm-dtd/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" specific-use="SMUR" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">EGUsphere</journal-id>
<journal-title-group>
<journal-title>EGUsphere</journal-title>
<abbrev-journal-title abbrev-type="publisher">EGUsphere</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">EGUsphere</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub"></issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/egusphere-2026-3271</article-id>
<title-group>
<article-title>Transport of anthropogenic CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt;-rich air from Asia across the North Pacific</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Woiwode</surname>
<given-names>Wolfgang</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Vogel</surname>
<given-names>Bärbel</given-names>
<ext-link>https://orcid.org/0000-0001-9763-3055</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lauther</surname>
<given-names>Valentin</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Grooß</surname>
<given-names>Jens-Uwe</given-names>
<ext-link>https://orcid.org/0000-0002-9485-866X</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Harrison</surname>
<given-names>Jeremy</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Johansson</surname>
<given-names>Sören</given-names>
<ext-link>https://orcid.org/0000-0002-9642-1955</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ungermann</surname>
<given-names>Jörn</given-names>
<ext-link>https://orcid.org/0000-0001-9095-8332</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Braesicke</surname>
<given-names>Peter</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dick</surname>
<given-names>Markus</given-names>
<ext-link>https://orcid.org/0000-0001-9278-4583</ext-link>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Engel</surname>
<given-names>Andreas</given-names>
<ext-link>https://orcid.org/0000-0003-0557-3935</ext-link>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Friedl-Vallon</surname>
<given-names>Felix</given-names>
<ext-link>https://orcid.org/0000-0003-2016-2800</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Glatthor</surname>
<given-names>Norbert</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gulde</surname>
<given-names>Thomas</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Höpfner</surname>
<given-names>Michael</given-names>
<ext-link>https://orcid.org/0000-0002-4174-9531</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Jesswein</surname>
<given-names>Markus</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
<xref ref-type="aff" rid="aff10">
<sup>10</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kaumanns</surname>
<given-names>Jan</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Keber</surname>
<given-names>Timo</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kleinert</surname>
<given-names>Anne</given-names>
<ext-link>https://orcid.org/0000-0003-3294-0278</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kretschmer</surname>
<given-names>Erik</given-names>
<ext-link>https://orcid.org/0000-0001-8923-5516</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Maucher</surname>
<given-names>Guido</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Neubert</surname>
<given-names>Tom</given-names>
<ext-link>https://orcid.org/0000-0001-8474-6560</ext-link>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Nordmeyer</surname>
<given-names>Hans</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Piesch</surname>
<given-names>Christof</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Plöger</surname>
<given-names>Felix</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Preusse</surname>
<given-names>Peter</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Retzlaff</surname>
<given-names>Markus</given-names>
<ext-link>https://orcid.org/0000-0002-8704-4211</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rhode</surname>
<given-names>Sebastian</given-names>
<ext-link>https://orcid.org/0000-0002-6070-9789</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rongen</surname>
<given-names>Heinz</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Schardt</surname>
<given-names>Georg</given-names>
<ext-link>https://orcid.org/0000-0001-7138-3502</ext-link>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Schuck</surname>
<given-names>Tanja</given-names>
<ext-link>https://orcid.org/0000-0002-1380-3684</ext-link>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
<xref ref-type="aff" rid="aff11">
<sup>11</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sinnhuber</surname>
<given-names>Björn-Martin</given-names>
<ext-link>https://orcid.org/0000-0001-9608-7320</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Strobel</surname>
<given-names>Johannes</given-names>
<ext-link>https://orcid.org/0009-0007-3457-6672</ext-link>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Trinkl</surname>
<given-names>Franziska</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff12">
<sup>12</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Van Luijt</surname>
<given-names>Ronja</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Versick</surname>
<given-names>Stefan</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Volk</surname>
<given-names>C. Michael</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wetzel</surname>
<given-names>Gerald</given-names>
<ext-link>https://orcid.org/0000-0002-6671-0297</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hoor</surname>
<given-names>Peter</given-names>
<ext-link>https://orcid.org/0000-0001-6582-6864</ext-link>
</name>
<xref ref-type="aff" rid="aff8">
<sup>8</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Riese</surname>
<given-names>Martin</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institute of Meteorology and Climate Research - Atmospheric Trace Gases and Remote Sensing (IMKASF), Karlsruhe  Institute of Technology, Karlsruhe, Germany</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institute of Climate and Energy Systems, Stratosphere (ICE-4), Forschungszentrum Jülich, Jülich, Germany</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>National Centre for Earth Observation, University of Leicester, Leicester, UK</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>School of Physics and Astronomy, University of Leicester, Leicester, UK</addr-line>
</aff>
<aff id="aff6">
<label>6</label>
<addr-line>Institute of Technology and Engineering (ITE), Forschungszentrum Jülich, Jülich, Germany</addr-line>
</aff>
<aff id="aff7">
<label>7</label>
<addr-line>Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, Frankfurt, Germany</addr-line>
</aff>
<aff id="aff8">
<label>8</label>
<addr-line>Johannes Gutenberg University of Mainz, Institute for Atmospheric Physics, Mainz, Germany</addr-line>
</aff>
<aff id="aff9">
<label>9</label>
<addr-line>now at: Cooperative Institute for Research in Environmental Sciences, University of Colorado-Boulder, Boulder, CO, USA</addr-line>
</aff>
<aff id="aff10">
<label>10</label>
<addr-line>now at: NOAA Earth System Research Laboratory Global Monitoring Division, Boulder, CO, USA</addr-line>
</aff>
<aff id="aff11">
<label>11</label>
<addr-line>now at: Centre for Isotope Research, University of Groningen, Groningen, the Netherlands</addr-line>
</aff>
<aff id="aff12">
<label>12</label>
<addr-line>now at: Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, Frankfurt, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>14</day>
<month>08</month>
<year>2026</year>
</pub-date>
<volume>2026</volume>
<fpage>1</fpage>
<lpage>34</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2026 Wolfgang Woiwode et al.</copyright-statement>
<copyright-year>2026</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2026/egusphere-2026-3271/">This article is available from https://egusphere.copernicus.org/preprints/2026/egusphere-2026-3271/</self-uri>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2026/egusphere-2026-3271/egusphere-2026-3271.pdf">The full text article is available as a PDF file from https://egusphere.copernicus.org/preprints/2026/egusphere-2026-3271/egusphere-2026-3271.pdf</self-uri>
<abstract>
<p>Dichloromethane (CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt;) is emitted mainly anthropogenically and suspected to delay stratospheric ozone recovery. We present in detail the first retrievals of mesoscale 2D distributions of CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; from infrared limb observations. The airborne remote sensing instrument GLORIA-AB (Gimballed Limb Observer for Radiance Imaging of the Atmosphere, hereinafter &amp;ldquo;GLORIA&amp;rdquo;) was deployed aboard the German research aircraft HALO during the PHILEAS campaign in August and September 2023 to study the outflow of the Asian Summer Monsoon (ASM). During long-range flights from Alaska, GLORIA observed filaments with elevated CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; above the North Pacific, Canada and Alaska. Filaments with horizontal extents along the flight track of up to ~1000 km and CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; volume mixing ratios of locally up to ~400 pptv were observed in the free troposphere, corresponding to levels more than six times higher than the northern hemispheric background for that season. Moderate CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; enhancements were detected locally also in air masses with characteristics of the extra-tropical lowermost stratosphere. We applied new high-resolution CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; spectroscopic data, resulting in ~11 % lower volume mixing ratios than in previous analyses using commonly available absorption cross sections. The GLORIA measurements are consistent with in situ observations on HALO by HAGAR-V and GhOST. Using back-trajectory analysis and surface-origin tracers by the CLaMS model, observed filaments are traced back to the ASM region and potential source regions are identified. Mesoscale filaments are shown to rapidly transport substantial amounts of CH&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;2&lt;/sub&gt; from the ASM across the North Pacific into the Northern Hemisphere Upper Troposphere and Lower Stratosphere (UTLS).</p>
</abstract>
<counts><page-count count="34"/></counts>
<funding-group>
<award-group id="gs1">
<funding-source>Deutsche Forschungsgemeinschaft</funding-source>
<award-id>316646266</award-id>
<award-id>VO 1276/7-1</award-id>
<award-id>HO 4120/4-1</award-id>
</award-group>
</funding-group>
</article-meta>
</front>
<body/>
<back>
</back>
</article>