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<front>
<journal-meta>
<journal-id journal-id-type="publisher">EGUsphere</journal-id>
<journal-title-group>
<journal-title>EGUsphere</journal-title>
<abbrev-journal-title abbrev-type="publisher">EGUsphere</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">EGUsphere</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub"></issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/egusphere-2025-3620</article-id>
<title-group>
<article-title>Prognostic simulations of mixed-phase clouds with model 1D-AC v1.0: The impact of freezing parameterizations on ice crystal budgets</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sun</surname>
<given-names>Yijia</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Fridlind</surname>
<given-names>Ann M.</given-names>
<ext-link>https://orcid.org/0000-0002-9020-0852</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Silber</surname>
<given-names>Israel</given-names>
<ext-link>https://orcid.org/0000-0001-6588-2145</ext-link>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Riemer</surname>
<given-names>Nicole</given-names>
<ext-link>https://orcid.org/0000-0002-3220-3457</ext-link>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Knopf</surname>
<given-names>Daniel A.</given-names>
<ext-link>https://orcid.org/0000-0001-7732-3922</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Stony Brook University, Stony Brook, NY 11794, USA</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>NASA Goddard Institute for Space Studies, New York, NY 10025, USA</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Pacific Northwest National Laboratory, Richland, WA 99352, USA</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>University of Illinois at Urbana-Champaign, Urbana, IL 61801, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>06</day>
<month>10</month>
<year>2025</year>
</pub-date>
<volume>2025</volume>
<fpage>1</fpage>
<lpage>48</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2025 Yijia Sun et al.</copyright-statement>
<copyright-year>2025</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2025/egusphere-2025-3620/">This article is available from https://egusphere.copernicus.org/preprints/2025/egusphere-2025-3620/</self-uri>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2025/egusphere-2025-3620/egusphere-2025-3620.pdf">The full text article is available as a PDF file from https://egusphere.copernicus.org/preprints/2025/egusphere-2025-3620/egusphere-2025-3620.pdf</self-uri>
<abstract>
<p>Mixed-phase clouds at high latitudes contribute to the uncertainty in predicting cloud feedbacks and climate sensitivity, mainly due to the complexity of microphysical processes that influence the partitioning between the supercooled liquid and ice phases, and hence, cloud radiative effects on regional scales. Particularly in Arctic mixed-phase clouds, the activation of ice-nucleating particles (INPs) from various aerosol populations remains a leading source of uncertainty. Our study employs a one-dimensional aerosol-cloud model informed by large-eddy simulations to probe the impact of INP representation on predicted ice crystal number concentrations (𝑁&lt;sub&gt;i&lt;/sub&gt;) and ice crystal budgets in mixed-phase Arctic stratus. We apply three immersion freezing (IMF) parameterizations, two time-independent (deterministic) and one time-dependent (classical nucleation theory), to predict the evolution of the INP reservoir and resulting ice crystal budget from polydisperse mineral dust, organic (humic-like substances), and sea spray aerosol particle size distributions. Our analysis focuses on how variations in aerosol number concentration and cloud system parameters such as cloud cooling rate, cloud-top entrainment rate, and ice crystal fall speed influence the INP reservoir and ice crystal budgets. Furthermore, this study investigates the competitive ice nucleation dynamics in mixed aerosol environments and provides a process-level quantification of the INP budget terms, which directly controls ice crystal budgets. For all studied case scenarios, the aerosol types and associated particle size distributions significantly impact INP and 𝑁&lt;sub&gt;i&lt;/sub&gt;, and the choice between a time-dependent and a deterministic freezing description yields orders-of-magnitude differences in the predicted INP and 𝑁&lt;sub&gt;i&lt;/sub&gt; over the 10 h simulation time, reflecting typical cloud lifetimes. Our results show that the influence of cloud cooling, INP entrainment, and sedimentation varies significantly depending on the chosen freezing parameterization. These findings underscore the critical need for robust IMF parameterizations and precise cloud system observations to enhance the accuracy of models in predicting mixed-phase cloud structure and evolution.</p>
</abstract>
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<funding-group>
<award-group id="gs1">
<funding-source>U.S. Department of Energy</funding-source>
<award-id>DE-SC0021034</award-id>
</award-group>
</funding-group>
</article-meta>
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