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<front>
<journal-meta>
<journal-id journal-id-type="publisher">EGUsphere</journal-id>
<journal-title-group>
<journal-title>EGUsphere</journal-title>
<abbrev-journal-title abbrev-type="publisher">EGUsphere</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">EGUsphere</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/egusphere-2023-2646</article-id>
<title-group>
<article-title>Diverse mixing state and ice nucleation properties of aerosol particles over the Western Pacific and the Southern Ocean</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Xue</surname>
<given-names>Jiao</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Zhang</surname>
<given-names>Tian</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Park</surname>
<given-names>Keyhong</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Yan</surname>
<given-names>Jinpei</given-names>
<ext-link>https://orcid.org/0000-0002-1273-9422</ext-link>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Yoon</surname>
<given-names>Young Jun</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Park</surname>
<given-names>Jiyeon</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wang</surname>
<given-names>Bingbing</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>State Key Laboratory of Marine Environmental Science, College of Ocean and Earth  Sciences, Xiamen University, Xiamen, 361102 China</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Korea Polar Research Institute, Incheon, 21990 South Korea</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Third Institute of Oceanography, Ministry of Natural Resources, Xiamen 361005,  China</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Center for Marine Meteorology and Climate Change, Xiamen University, Xiamen,  361102 China</addr-line>
</aff>
<pub-date pub-type="epub">
<day>13</day>
<month>11</month>
<year>2023</year>
</pub-date>
<volume>2023</volume>
<fpage>1</fpage>
<lpage>51</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2023 Jiao Xue et al.</copyright-statement>
<copyright-year>2023</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2023/egusphere-2023-2646/">This article is available from https://egusphere.copernicus.org/preprints/2023/egusphere-2023-2646/</self-uri>
<self-uri xlink:href="https://egusphere.copernicus.org/preprints/2023/egusphere-2023-2646/egusphere-2023-2646.pdf">The full text article is available as a PDF file from https://egusphere.copernicus.org/preprints/2023/egusphere-2023-2646/egusphere-2023-2646.pdf</self-uri>
<abstract>
<p>Atmospheric particles from different sources can impact cloud formation and play a critical role in regulating cloud properties. However, particle characteristics at single particle level and their abilities to serve as ice nucleating particles (INPs) over different marine atmosphere are poorly understood. Here, we present characterizations and ice nucleation properties of particles collected during a northern and southern hemisphere cruise from South Korea to Antarctica. Micro-spectroscopic analysis was used to obtain composition of individual particles and mixing state of particle populations. Major particle classes were identified and have different contributions over the Western Pacific and the Southern Ocean, including fresh and aged sea salt, sea salt mixed with sulfate, carbonaceous, sulfur-containing, and dust particles. Increasing contribution of fresh sea salt particles, the dominate particle class in the samples, tended toward an increasing mixing state index indicating the population becoming more internally mixed. Aging processes and new particle sources introduce particles with new compositions resulting in external mixtures. We found that the investigated particles demonstrated a variety of ice nucleation abilities at cirrus conditions. The identified INPs are all major particle classes present in the population, and the sea salt mixed sulfate particle is enriched in INPs. Aging processes affected both particle mixing state and their ice nucleation abilities. We tested different ice nucleation parameterizations of marine atmospheric particles for their applicability. Finally, we discuss how the mixing state of particle populations impacts ice nucleation in the atmosphere.</p>
</abstract>
<counts><page-count count="51"/></counts>
<funding-group>
<award-group id="gs1">
<funding-source>National Natural Science Foundation of China</funding-source>
<award-id>42075076</award-id>
<award-id>41775133</award-id>
</award-group>
<award-group id="gs2">
<funding-source>Fundamental Research Funds for the Central Universities</funding-source>
<award-id>20720160111</award-id>
<award-id>20720190147</award-id>
</award-group>
<award-group id="gs3">
<funding-source>Korea Polar Research Institute</funding-source>
<award-id>PE24110</award-id>
<award-id>PE24030</award-id>
</award-group>
<award-group id="gs4">
<funding-source>Key Laboratory of Global Change and Marine-Atmospheric Chemistry</funding-source>
<award-id>GCMAC2004</award-id>
</award-group>
</funding-group>
</article-meta>
</front>
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